↩ Accueil

Vue lecture

Coulomb liquid emerges from five electrons in a semiconductor

As few as five electrons in a semiconductor can exhibit collective behaviour, forming a “Coulomb liquid”, according to researchers in Europe. This extends the study of correlated systems to electron plasmas, and could lead to the study of other exotic phases of matter.

A conventional plasma is a hot, ionized gas of free electrons and positive ions. However, the conduction band of a semiconductor can be considered a one-component plasma. “The effect of the positive charges, as they are locked into the lattice, can be modelled as a uniform background of positive charge,” says team member Vyacheslavs Kashcheyevs of the University of Latvia in Riga. In conventional electronics and semiconductor physics, the conduction band is modelled as a 2D Fermi gas of non-interacting particles, with the Coulomb interaction between the electrons neglected.

The new work focused on electron–electron correlations in the conduction band of gallium arsenide at millikelvin temperatures. The team created a Y-shaped junction. Electrons emitted from a quantum dot were steered through the device by an externally-generated surface acoustic wave (SAW) potential. Part-way through, the path divided, and each electron could either go left or right. The number taking each path was measured by separate quantum dots. The researchers are uncertain, and the model is agnostic, about the extent to which the randomness of left or right arose from quantum mechanics.

When no more than one electron was loaded into each potential minimum, each electron’s choice was random, and the number of electrons counted at each detector after multiple trials could be modelled by a binomial distribution. However, when the researchers tuned the apparatus such that each minimum contained multiple electrons, they found changes in the distribution, with groups of particles less likely to travel to the same detector than would be naïvely expected.

Calculating “cumulants”

The researchers quantified the changes in the distributions using probability theory, calculating “cumulants” of the distributions. “We not only have a cumulant of order two, which would say that two particles are repulsing,” says Hermann Sellier of Institut Néel in Grenoble, France, who led the experimental research. “We have a cumulant of order four for four particles or five for five particles, showing that each particle is talking to all the other particles of the droplet. That’s much stronger and something that has not been measured before.”

This shows, say the researchers, that the 2D electron gas condenses into a strongly correlated Coulomb liquid. This a phase of matter seen in quark–gluon plasma, which is created by the high-energy collision of heavy ions, but never previously identified in electronic matter.

“It’s not like you have atoms which, below a certain temperature, go from the gas phase to the liquid phase because of an attractive interaction,” explains Sellier. “We say that the correlated behaviour is like that of a liquid, but a very special liquid made of repulsive interactions. You push on the right, it pushes on the left.” This is possible only at low temperatures because heating increases the entropy to the point where the correlated state of matter is disfavoured.

The team now wants to look at larger systems approaching the macroscopic limit. They believe similar systems could potentially be used to study many-body physics with other, exotic particles such as anyons – quasiparticles that have properties intermediate to bosons and fermions. Potential technological applications include cold atom quantum simulation.

Considerable interest

Ravi Rau of Louisiana State University in the US says, “It is an interesting method, novel to me, of controlling electron droplets and being able to measure correlations of two, three and up to a maximum of five-particles so far, and addressing the general question of the transition in few-body systems to the statistical limit from explicit dynamics when the number of particles is small”. He adds, “This study, such a system, and the results presented will of course be of considerable interest.”

Rau does however, note that very similar results were achieved in the past in studies of electron collisions with cold atoms and molecules. “[That technique] went under the name of COLTRIMS (cold target recoil-ion momentum spectroscopy) allowed measuring multiple differential cross sections and studying electron–electron correlations in atoms,” he says. “It was the exact analogue of this [work], except that instead of an artificially created and controlled droplet cluster, the electrons were naturally inside the atom.”

The researchers acknowledge the similarity, and thank Rau for bringing the previous work to their attention. However, Kashcheyevs argues that the new work has a generality that allows it to tackle new problems, finding the scaling law that connects the properties of individual electrons to the properties of incompressible Coulomb plasma. “Applying our method at lower temperatures in the future can probe the quantum regime of the phase diagram of this electronic fluid, which is known to support exotic quasiparticles impossible in the 3D vacuum of the Standard Model,” he says.

The research is described in Nature.

The post Coulomb liquid emerges from five electrons in a semiconductor appeared first on Physics World.

  •  

Quantum twisting microscope measures phasons in cryogenic graphene

By adapting their quantum twisting microscope to operate at cryogenic temperatures, researchers have made the first observations of a type of phonon that occurs in twisted bilayer graphene.  These “phasons” could have implications for the electron dynamics in these materials.

Graphene is a layer of carbon just one atom thick and it has range of fascinating and useful properties – as do bilayer and multilayer versions of graphene. Since 2018, condensed-matter physicists have been captivated by the intriguing electron behaviour in two layers of graphene that are rotated with respect to each other.

As the twist angle deviates from zero, the bilayer becomes a moiré superlattice. The emergence of this structure influences electronic properties of the material, which can transform from a semiconductor to a superconductor.

In 2023, researchers led by Shahal Ilani at the Weizmann Institute of Science in Israel developed a quantum twisting microscope to study these effects. Based on a scanning probe microscope with graphene on the substrate and folded over the tip such as to give it a flat end, the instrument allows precise control over the relative orientation between two graphene surfaces – in particular, the twist angle.

Strange metals

Now Ilani and an international team have operated the microscope at cryogenic temperatures for the first time. So far, their measurements support the current understanding of how electrons couple to phasons, which are specific modes of phonons (quantized lattice vibrations). Characterizing this coupling could help us understand “strange metals”, whose electrical resistance increases at lower temperatures – which is the opposite of normal metals.

There are different types of phonons, such as acoustic phonons where atoms within the same unit cell oscillate in phase with each other, and optical phonons where they oscillate out of phase. Phasons are phonons involving lattice oscillations in one layer that are out of phase or antisymmetric with oscillations in the layer above.

“This is the one that turns out to be very important for how the electrons behave between the layers because even a small relative displacement between the two layers affects how the electrons go from one layer to the other,” explains Weizmann’s John Birkbeck as he describes the role of phasons in twisted bilayer graphene materials.

For most phonons the coupling to electrons is weaker the lower the energy of the phonon mode. However for twisted bilayer materials, theory suggests that phason coupling to electrons increases as the twist between the two layers approaches alignment due to the antisymmetric motion of the two layers and the heightened sensitivity of interlayer tunnelling to small relative displacements.

Unique perspective

“There are not that many tools to see phonons, particularly in moiré systems” adds Birkbeck. This is where the quantum twisting microscope offers a unique perspective. Thanks to the atomically flat end of the tip, electrons can tunnel between the layer on the substrate and the layer on the tip whenever there is a matching state in terms of not just energy but also momentum too.

Where there is a momentum mismatch, tunnelling between tip and substrate is still possible by balancing the mismatch with the emission or absorption of a phonon. By operating at cryogenic temperatures, the researchers were able to get a measure of these momentum transactions and probe the electron phonon coupling too.

“What was interesting from this work is not only that we could image the phonon dispersion, but also we can quantify it,” says Birkbeck stressing the absolute nature of these quantified electron phonon coupling-strength measurements.

The measurements are the first observations of phasons in twisted bilayer graphene and reveal a strong increase in coupling as the layers approach alignment, as predicted by theory. However, the researchers were not able to study angles smaller than 6°. Below this angle the tunnelling resistance is so low that the contact resistance starts to warp readings, among other limiting factors.

Navigating without eyes

A certain amount of technical adjustment was needed to operate the tool at cryogenic temperatures, not least to “to navigate without eyes” because the team was not able to incorporate their usual optics with the cryogenic set up. The researchers hope that with further technical adjustments they will be able to use the quantum twisting microscope in cryogenic conditions at the magic angle of 1.1°, where superconductivity occurs.

Pablo Jarillo Herrero, who led the team at MIT that first reported superconductivity in twisted bilayer graphene in 2018 but was not involved in this research describes it as an “interesting study” adding, “I’m looking forward to seeing more interesting results from low temperature QTM research!”

Hector Ochoa De Eguileor Romillo at Columbia University in the US, who proposed a role for phason–electron interactions in these materials in 2019, but was also not involved in this research describes it as “a beautiful experiment”. He adds, “I think it is fair to say that this is the most exciting experimental technique of the last 15 years or so in condensed matter physics; new interesting data are surely coming.”

The research is described in Nature.

The post Quantum twisting microscope measures phasons in cryogenic graphene appeared first on Physics World.

  •  

Superconducting device delivers ultrafast changes in magnetic field

Precise control over the generation of intense, ultrafast changes in magnetic fields called “magnetic steps” has been achieved by researchers in Hamburg, Germany. Using ultrashort laser pulses, Andrea Cavalleri and colleagues at the Max Planck Institute for the Structure and Dynamics of Matter disrupted the currents flowing through a superconducting disc. This alters the superconductor’s local magnetic environment on very short timescales – creating a magnetic step.

Magnetic steps rise to their peak intensity in just a few picoseconds, before decaying more slowly in several nanoseconds. They are useful to scientists because they rise and fall on timescales far shorter than the time it takes for materials to respond to external magnetic fields. As a result, magnetic steps could provide fundamental insights into the non-equilibrium properties of magnetic materials, and could also have practical applications in areas such as magnetic memory storage.

So far, however, progress in this field has been held back by technical difficulties in generating and controlling magnetic steps on ultrashort timescales. Previous strategies  have employed technologies including microcoils, specialized antennas, and circularly polarized light pulses. However, each of these schemes offer a limited degree of control over the properties of the magnetic steps they generated.

Quenching supercurrents

Now, Cavalleri’s team has developed a new technique that involves the quenching of currents in a superconductor. Normally, these “supercurrents” will flow indefinitely without losing energy, and will act to expel any external magnetic fields from the superconductor’s interior. However, if these currents are temporarily disrupted on ultrashort timescales, a sudden change will be triggered in the magnetic field close to the superconductor – which could be used to create a magnetic step.

To create this process, Cavalleri and colleagues applied ultrashort laser pulses to a thin, superconducting disc of yttrium barium copper oxide (YBCO), while also exposing the disc to an external magnetic field.

To detect whether magnetic steps had been generated, they placed a crystal of the semiconductor gallium phosphide in the superconductor’s vicinity. This material exhibits an extremely rapid Faraday response. This involves the rotation of the polarization of light passing through the semiconductor in response to changes in the local magnetic field. Crucially, this rotation can occur on sub-picosecond timescales.

In their experiments, researchers monitored changes to the polarization of an ultrashort “probe” laser pulse passing through the semiconductor shortly after they quenched supercurrents in their YBCO disc using a separate ultrashort “pump” laser pulse.

“By abruptly disrupting the material’s supercurrents using ultrashort laser pulses, we could generate ultrafast magnetic field steps with rise times of approximately one picosecond – or one trillionth of a second,” explains team member Gregor Jotzu.

Broadband step

This was used to generate an extremely broadband magnetic step, which contains frequencies ranging from sub-gigahertz to terahertz. In principle, this should make the technique suitable for studying magnetization in a diverse variety of materials.

To demonstrate practical applications, the team used these magnetic steps to control the magnetization of a ferrimagnet. Such a magnet has opposing magnetic moments, but has a non-zero spontaneous magnetization in zero magnetic field.

When they placed a ferrimagnet on top of their superconductor and created a magnetic step, the step field caused the ferrimagnet’s magnetization to rotate.

For now, the magnetic steps generated through this approach do not have the speed or amplitude needed to switch materials like a ferrimagnet between stable states. Yet through further tweaks to the geometry of their setup, the researchers are confident that this ability may not be far out of reach.

“Our goal is to create a universal, ultrafast stimulus that can switch any magnetic sample between stable magnetic states,” Cavalleri says. “With suitable improvements, we envision applications ranging from phase transition control to complete switching of magnetic order parameters.”

The research is described in Nature Photonics.

The post Superconducting device delivers ultrafast changes in magnetic field appeared first on Physics World.

  •